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Abstract. Climate models predict that the Brewer–Dobson circulation (BDC) will accelerate due to tropospheric warming, leading to a redistribution of trace gases and, consequently, to a change of the radiative properties of the atmosphere. Changes in the BDC are diagnosed by the so-called “age of air”, that is, the time since air in the stratosphere exited the troposphere. These changes can be derived from a long-term observation-based record of long-lived trace gases with increasing concentration in the troposphere, such as sulfur hexafluoride (SF6). The Atmospheric Chemistry Experiment Fourier Transform Spectrometer (ACE-FTS) provides the longest available continuous time series of vertically resolved SF6 measurements, spanning 2004 to the present. In this study, a new age-of-air product is derived from the ACE-FTS SF6 dataset. The ACE-FTS product is in good agreement with other observation-based age-of-air datasets and shows the expected global distribution of age-of-air values. Age of air from a chemistry–climate model is evaluated, and the linear trend of the observation-based age of air is calculated in 12 regions within the lower stratospheric midlatitudes (14–20 km, 40–70°) in each hemisphere. In 8 of 12 regions, there was not a statistically significant trend. The trends in the other regions, specifically 50–60 and 60–70° S at 17–20 km and 40–50° N at 14–17 and 17–20 km, are negative and significant to 2 standard deviations. This is therefore the first observation-based age-of-air trend study to suggest an acceleration of the shallow branch of the BDC, which transports air poleward in the lower stratosphere, in regions within both hemispheres. 

Abstract The age of seawater refers to the amount of time that has elapsed since that water encountered the surface. This age measures the ventilation rate of the ocean, and the spatial distribution of age can be influenced by multiple processes, such as overturning circulation, ocean mixing, and air–sea exchange. In this work, we aim to gain new quantitative insights about how the ocean’s age tracer distribution reflects the strength of the meridional overturning circulation and diapycnal diffusivity. We propose an integral constraint that relates the age tracer flow across an isopycnal surface to the geometry of the surface. With the integral constraint, a relationship between the globally averaged effective diapycnal diffusivity and the meridional overturning strength at an arbitrary density level can be inferred from the age tracer concentration near that level. The theory is tested in a set of idealized single-basin simulations. A key insight from this study is that the age difference between regions of upwelling and downwelling, rather than any single absolute age value, is the best indicator of overturning strength. The framework has also been adapted to estimate the strength of abyssal overturning circulation in the modern North Pacific, and we demonstrate that the age field provides an estimate of the circulation strength consistent with previous studies. This framework could potentially constrain ocean circulation and mixing rates from age-like realistic tracers (e.g., radiocarbon) in both past and present climates. Significance StatementThe age of seawater—the local mean time since local water from different pathways was last at the surface—is a valuable indicator of ocean circulation and the transport time scale of heat and carbon. We introduce a novel constraint that relates total age flow across a density surface to its geometry, which provides new insights into constraining ocean circulation and mixing rates from age-like realistic tracers (e.g., radiocarbon). 

Abstract The nonnormality of temperature probability distributions and the physics that drive it are important due to their relationships to the frequency of extreme warm and cold events. Here we use a conditional mean framework to explore how horizontal temperature advection and other physical processes work together to control the shape of daily temperature distributions during 1979–2019 in the ERA5 dataset for both JJA and DJF. We demonstrate that the temperature distribution in the middle and high latitudes can largely be linearly explained by the conditional mean horizontal temperature advection with the simple treatment of other processes as a Newtonian relaxation with a spatially variant relaxation time scale and equilibrium temperature. We analyze the role of different transient and stationary components of the horizontal temperature advection in affecting the shape of temperature distributions. The anomalous advection of the stationary temperature gradient has a dominant effect in influencing temperature variance, while both that term and the covariance between anomalous wind and anomalous temperature have significant effects on temperature skewness. While this simple method works well over most of the ocean, the advection–temperature relationship is more complicated over land. We classify land regions with different advection–temperature relationships under our framework, and find that for both seasons the aforementioned linear relationship can explain ∼30% of land area, and can explain either the lower or the upper half of temperature distributions in an additional ∼30% of land area. Identifying the regions where temperature advection explains shapes of temperature distributions well will help us gain more confidence in understanding the future change of temperature distributions and extreme events. 

Abstract Wave‐induced adiabatic mixing in the winter midlatitudes is one of the key processes impacting stratospheric transport. Understanding its strength and structure is vital to understanding the distribution of trace gases and their modulation under a changing climate. Age‐of‐air is often used to understand stratospheric transport, and this study proposes refinements to the vertical age gradient theory of Linz et al. (2021),https://doi.org/10.1029/2021JD035199. The theory assumes exchange of air between a well‐mixed tropics and a well‐mixed extratropics, separated by a transport barrier, quantifying the adiabatic mixing flux across the interface using age‐based measures. These assumptions are re‐evaluated and a refined framework that includes the effects of meridional tracer gradients is established to quantify the mixing flux. This is achieved, in part, by computing a circulation streamfunction in age‐potential temperature coordinates to generate a complete distribution of parcel ages being mixed in the midlatitudes. The streamfunction quantifies the “true” age of parcels mixed between the tropics and the extratropics. Applying the revised theory to an idealized and a comprehensive climate model reveals that ignoring the meridional gradients in age leads to an underestimation of the wave‐driven mixing flux. Stronger, and qualitatively similar fluxes are obtained in both models, especially in the lower‐to‐middle stratosphere. While the meridional span of adiabatic mixing in the two models exhibits some differences, they show that the deep tropical pipe, that is, latitudes equatorward of 15° barely mix with older midlatitude air. The novel age‐potential temperature circulation can be used to quantify additional aspects of stratospheric transport.